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ContentControl.Ungroup Method

Removes a group content control from a document so that its child content controls are no longer nested and can be freely edited.

Namespace:  Microsoft.Office.Interop.Word
Assembly:  Microsoft.Office.Interop.Word (in Microsoft.Office.Interop.Word.dll)

void Ungroup()

This method fails if you run it on a control that is not of type wdContentControlGroup.